Detection of aerosol particles from siberian biomass burning over the western north pacific

Momoka Yoshizue, Fumikazu Taketani, Kouji Adachi, Yoko Iwamoto, Yasunori Tohjima, Tatsuhiro Mori, Kazuhiko Miura

Research output: Contribution to journalArticlepeer-review

3 Citations (Scopus)

Abstract

Carbonaceous aerosol particles emitted from biomass burning (BB) have a large impact on the global climate. In particular, tarball particles (TBs), which are spherical organic aerosol particles, account for a large proportion of aerosol particles from BB. In this study, we collected aerosol particles over the western North Pacific and analyzed them using transmission electron microscopy with energy-dispersive X-ray spectroscopy (TEM-EDX) to reveal their shape and composition. We detected TBs and organic carbon particles originating from Siberian forest fires. To the best of our knowledge, this is the first case in which a large number of TBs have been found over the Pacific Ocean far from the BB source. The spherical shapes of the TBs were maintained even after long-range transport. In addition, our individual analysis of TBs showed that the size and composition of TBs differ depending on the air mass origin. The occurrence and microphysical properties of TBs are important to accurately evaluate the impact of TBs on climate. Our results imply that TBs can be transported to the Arctic and have an influence on radiative forcing over the ocean and in the Arctic.

Original languageEnglish
Article number1175
JournalAtmosphere
Volume11
Issue number11
DOIs
Publication statusPublished - 2020 Nov
Externally publishedYes

Keywords

  • Individual particle analysis
  • Pacific Ocean
  • Tarball

ASJC Scopus subject areas

  • Environmental Science (miscellaneous)

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