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Heterogeneous synergistic catalysis by a palladium complex and an amine on a silica surface for acceleration of the Tsuji-Trost reaction

  • Hiroto Noda
  • , Ken Motokura
  • , Akimitsu Miyaji
  • , Toshihide Baba

Research output: Contribution to journalArticlepeer-review

Abstract

The cooperative surface-catalysis strategy of a Brønsted acid and an organic base can be extended to a metal complex and organic base pair. A silica-supported diaminopalladium complex and a tertiary amine were prepared and characterized. The Pd-catalyzed Tsuji-Trost reaction was enhanced significantly by the presence of the tertiary amine on the same silica surface as the Pd complex.

Original languageEnglish
Pages (from-to)8017-8020
Number of pages4
JournalAngewandte Chemie - International Edition
Volume51
Issue number32
DOIs
Publication statusPublished - 2012 Aug 6
Externally publishedYes

Keywords

  • amines
  • heterogeneous catalysis
  • palladium
  • supported catalysis
  • Tsuji-Trost reaction

ASJC Scopus subject areas

  • Catalysis
  • General Chemistry

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