Non-Markovian effects of intermolecular vibrational coherence on femtosecond time-resolved coherent anti-Stokes Raman scattering from molecules in condensed phases

M. Sugawara; M. Hayashi; Y. Fujimura

doi:10.1016/0009-2614(92)85213-T

Non-Markovian effects of intermolecular vibrational coherence on femtosecond time-resolved coherent anti-Stokes Raman scattering from molecules in condensed phases

M. Sugawara, M. Hayashi, Y. Fujimura

Department of Chemistry

Research output: Contribution to journal › Article › peer-review

Abstract

Non-Markovian effects of intermolecular vibrational coherences on femtosecond time-resolved coherent anti-Stokes Raman scattering (CARS) from a molecular mixture are theoretically studied. The non-Markovian behavior of intermolecular vibrational coherence transfers based on a stochastic model results in the suppresion of the frequency shifts of quantum beats in the time-resolved CARS profiles compared with the case in the Markovian approximation.

Original language	English
Pages (from-to)	346-352
Number of pages	7
Journal	Chemical Physics Letters
Volume	189
Issue number	4-5
DOIs	https://doi.org/10.1016/0009-2614(92)85213-T
Publication status	Published - 1992 Feb 14

ASJC Scopus subject areas

Physics and Astronomy(all)
Physical and Theoretical Chemistry

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10.1016/0009-2614(92)85213-T

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title = "Non-Markovian effects of intermolecular vibrational coherence on femtosecond time-resolved coherent anti-Stokes Raman scattering from molecules in condensed phases",

abstract = "Non-Markovian effects of intermolecular vibrational coherences on femtosecond time-resolved coherent anti-Stokes Raman scattering (CARS) from a molecular mixture are theoretically studied. The non-Markovian behavior of intermolecular vibrational coherence transfers based on a stochastic model results in the suppresion of the frequency shifts of quantum beats in the time-resolved CARS profiles compared with the case in the Markovian approximation.",

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AU - Hayashi, M.

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PY - 1992/2/14

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N2 - Non-Markovian effects of intermolecular vibrational coherences on femtosecond time-resolved coherent anti-Stokes Raman scattering (CARS) from a molecular mixture are theoretically studied. The non-Markovian behavior of intermolecular vibrational coherence transfers based on a stochastic model results in the suppresion of the frequency shifts of quantum beats in the time-resolved CARS profiles compared with the case in the Markovian approximation.

AB - Non-Markovian effects of intermolecular vibrational coherences on femtosecond time-resolved coherent anti-Stokes Raman scattering (CARS) from a molecular mixture are theoretically studied. The non-Markovian behavior of intermolecular vibrational coherence transfers based on a stochastic model results in the suppresion of the frequency shifts of quantum beats in the time-resolved CARS profiles compared with the case in the Markovian approximation.

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Non-Markovian effects of intermolecular vibrational coherence on femtosecond time-resolved coherent anti-Stokes Raman scattering from molecules in condensed phases

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