Suppression of intramolecular vibrational energy redistribution by intense CW-laser fields

M. Sugawara

doi:10.1155/2011/584082

Suppression of intramolecular vibrational energy redistribution by intense CW-laser fields

M. Sugawara

Department of Chemistry

Research output: Contribution to journal › Article › peer-review

2 Citations (Scopus)

Abstract

We present a quantum control scheme which realizes suppression of the intramolecular vibrational energy redistribution (IVR). In this scheme, we utilize effective decomposition brought by intense CW-laser fields, which enables to exclude the doorway state coupled to background manifolds. In doing so, we introduce a helper state and make it optically coupled with the doorway state through the intense CW-laser field. We have applied the present scheme to both the Bixon-Jortner model and the SCCl2 model system.

Original language	English
Article number	584082
Journal	Advances in Physical Chemistry
Volume	2011
DOIs	https://doi.org/10.1155/2011/584082
Publication status	Published - 2011

ASJC Scopus subject areas

Physical and Theoretical Chemistry

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abstract = "We present a quantum control scheme which realizes suppression of the intramolecular vibrational energy redistribution (IVR). In this scheme, we utilize effective decomposition brought by intense CW-laser fields, which enables to exclude the doorway state coupled to background manifolds. In doing so, we introduce a helper state and make it optically coupled with the doorway state through the intense CW-laser field. We have applied the present scheme to both the Bixon-Jortner model and the SCCl2 model system.",

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AB - We present a quantum control scheme which realizes suppression of the intramolecular vibrational energy redistribution (IVR). In this scheme, we utilize effective decomposition brought by intense CW-laser fields, which enables to exclude the doorway state coupled to background manifolds. In doing so, we introduce a helper state and make it optically coupled with the doorway state through the intense CW-laser field. We have applied the present scheme to both the Bixon-Jortner model and the SCCl2 model system.

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Suppression of intramolecular vibrational energy redistribution by intense CW-laser fields

Abstract

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