An access to the 13-membered cyclophane substructure in GKK1032AS: An intramolecular 1,4-addition approach

Satoka Nagai; Yuka Yamagishi; Yuta Shimizu; Ken Ichi Takao; Kin Ichi Tadano

doi:10.3987/COM-14-S(K)55

An access to the 13-membered cyclophane substructure in GKK1032AS: An intramolecular 1,4-addition approach

Satoka Nagai, Yuka Yamagishi, Yuta Shimizu, Ken Ichi Takao, Kin Ichi Tadano

応用化学科

研究成果: Article › 査読

5 被引用数 (Scopus)

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The construction of the 13-membered para-cyclophane substructure in GKK1032As, a member of novel pyrrolidinone-containing bioactive natural products, has been explored. An efficient approach for this synthetically formidable object was found, which relied on an intramolecular 1,4-addition between a nitromethylene group and a vinyl ketone moiety both incorporated as side chains into the 6/5/6-tricyclic (the A/B/C-ring system) of the GKK1032s.

本文言語	English
ページ（範囲）	819-826
ページ数	8
ジャーナル	Heterocycles
巻	90
号	2
DOI	https://doi.org/10.3987/COM-14-S(K)55
出版ステータス	Published - 2015

ASJC Scopus subject areas

分析化学
薬理学
有機化学

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10.3987/COM-14-S(K)55

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abstract = "The construction of the 13-membered para-cyclophane substructure in GKK1032As, a member of novel pyrrolidinone-containing bioactive natural products, has been explored. An efficient approach for this synthetically formidable object was found, which relied on an intramolecular 1,4-addition between a nitromethylene group and a vinyl ketone moiety both incorporated as side chains into the 6/5/6-tricyclic (the A/B/C-ring system) of the GKK1032s.",

author = "Satoka Nagai and Yuka Yamagishi and Yuta Shimizu and Takao, {Ken Ichi} and Tadano, {Kin Ichi}",

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language = "English",

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AU - Nagai, Satoka

AU - Yamagishi, Yuka

AU - Shimizu, Yuta

AU - Takao, Ken Ichi

AU - Tadano, Kin Ichi

PY - 2015

Y1 - 2015

N2 - The construction of the 13-membered para-cyclophane substructure in GKK1032As, a member of novel pyrrolidinone-containing bioactive natural products, has been explored. An efficient approach for this synthetically formidable object was found, which relied on an intramolecular 1,4-addition between a nitromethylene group and a vinyl ketone moiety both incorporated as side chains into the 6/5/6-tricyclic (the A/B/C-ring system) of the GKK1032s.

AB - The construction of the 13-membered para-cyclophane substructure in GKK1032As, a member of novel pyrrolidinone-containing bioactive natural products, has been explored. An efficient approach for this synthetically formidable object was found, which relied on an intramolecular 1,4-addition between a nitromethylene group and a vinyl ketone moiety both incorporated as side chains into the 6/5/6-tricyclic (the A/B/C-ring system) of the GKK1032s.

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VL - 90

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JO - Heterocycles

JF - Heterocycles

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An access to the 13-membered cyclophane substructure in GKK1032AS: An intramolecular 1,4-addition approach

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