Non-Markovian effects of intermolecular vibrational coherence on femtosecond time-resolved coherent anti-Stokes Raman scattering from molecules in condensed phases

M. Sugawara; M. Hayashi; Y. Fujimura

doi:10.1016/0009-2614(92)85213-T

Non-Markovian effects of intermolecular vibrational coherence on femtosecond time-resolved coherent anti-Stokes Raman scattering from molecules in condensed phases

M. Sugawara, M. Hayashi, Y. Fujimura

化学科

研究成果: Article › 査読

抄録

Non-Markovian effects of intermolecular vibrational coherences on femtosecond time-resolved coherent anti-Stokes Raman scattering (CARS) from a molecular mixture are theoretically studied. The non-Markovian behavior of intermolecular vibrational coherence transfers based on a stochastic model results in the suppresion of the frequency shifts of quantum beats in the time-resolved CARS profiles compared with the case in the Markovian approximation.

本文言語	English
ページ（範囲）	346-352
ページ数	7
ジャーナル	Chemical Physics Letters
巻	189
号	4-5
DOI	https://doi.org/10.1016/0009-2614(92)85213-T
出版ステータス	Published - 1992 2月 14

ASJC Scopus subject areas

物理学および天文学（全般）
物理化学および理論化学

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10.1016/0009-2614(92)85213-T

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引用スタイル

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