Photoelectron spectroscopy and mass distributions of aluminum-sulfur cluster anions (AlnSm-)

Atsushi Nakajima; Nan Zhang; Hiroshi Kawamata; Takasuke Hayase; Kojiro Nakao; Koji Kaya

doi:10.1016/0009-2614(95)00653-L

Photoelectron spectroscopy and mass distributions of aluminum-sulfur cluster anions (Al_nS_m^-)

Atsushi Nakajima
, Nan Zhang
, Hiroshi Kawamata
, Takasuke Hayase
, Kojiro Nakao
, Koji Kaya

化学科

研究成果: Article › 査読

15 被引用数 (Scopus)

抄録

Photoelectron spectra of Al_nS_m^- cluster anions (0 ≤ n, m ≤ 10) were measured at photon energies of 3.49 and 4.66 eV, by using a magnetic bottle electron spectrometer. The Al_nS_m^-. clusters were produced by laser vaporization of an aluminum-sulfur mixed rod in He carrier gas. The abundant AI_nSM clusters are three types of AlS^-(Al₂S₃)_k, AlS₂^-(Al₂S₃)_k, and (Al₂S₃)_k^-, where an unit of Al₂S₃ aggregates with ion cores of AlS^-, AlS₂^-, and Al₂S₃, respectively. Al₃S₃ is exceptionally stable with its geometrical structure.

本文言語	English
ページ（範囲）	295-300
ページ数	6
ジャーナル	Chemical Physics Letters
巻	241
号	4
DOI	https://doi.org/10.1016/0009-2614(95)00653-L
出版ステータス	Published - 1995 7月 28

ASJC Scopus subject areas

物理学および天文学一般
物理化学および理論化学

文献へのアクセス

10.1016/0009-2614(95)00653-L

他のファイルとリンク

引用スタイル

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title = "Photoelectron spectroscopy and mass distributions of aluminum-sulfur cluster anions (AlnSm-)",

abstract = "Photoelectron spectra of AlnSm- cluster anions (0 ≤ n, m ≤ 10) were measured at photon energies of 3.49 and 4.66 eV, by using a magnetic bottle electron spectrometer. The AlnSm-. clusters were produced by laser vaporization of an aluminum-sulfur mixed rod in He carrier gas. The abundant AInSM clusters are three types of AlS-(Al2S3)k, AlS2-(Al2S3)k, and (Al2S3)k-, where an unit of Al2S3 aggregates with ion cores of AlS-, AlS2-, and Al2S3, respectively. Al3S3 is exceptionally stable with its geometrical structure.",

author = "Atsushi Nakajima and Nan Zhang and Hiroshi Kawamata and Takasuke Hayase and Kojiro Nakao and Koji Kaya",

note = "Funding Information: work was partly supported by a Grant-in-Aid for Scientific Research on Priority Areas from the Ministry of Education, Science and Culture.",

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doi = "10.1016/0009-2614(95)00653-L",

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AU - Nakajima, Atsushi

AU - Zhang, Nan

AU - Kawamata, Hiroshi

AU - Hayase, Takasuke

AU - Nakao, Kojiro

AU - Kaya, Koji

N1 - Funding Information: work was partly supported by a Grant-in-Aid for Scientific Research on Priority Areas from the Ministry of Education, Science and Culture.

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Y1 - 1995/7/28

N2 - Photoelectron spectra of AlnSm- cluster anions (0 ≤ n, m ≤ 10) were measured at photon energies of 3.49 and 4.66 eV, by using a magnetic bottle electron spectrometer. The AlnSm-. clusters were produced by laser vaporization of an aluminum-sulfur mixed rod in He carrier gas. The abundant AInSM clusters are three types of AlS-(Al2S3)k, AlS2-(Al2S3)k, and (Al2S3)k-, where an unit of Al2S3 aggregates with ion cores of AlS-, AlS2-, and Al2S3, respectively. Al3S3 is exceptionally stable with its geometrical structure.

AB - Photoelectron spectra of AlnSm- cluster anions (0 ≤ n, m ≤ 10) were measured at photon energies of 3.49 and 4.66 eV, by using a magnetic bottle electron spectrometer. The AlnSm-. clusters were produced by laser vaporization of an aluminum-sulfur mixed rod in He carrier gas. The abundant AInSM clusters are three types of AlS-(Al2S3)k, AlS2-(Al2S3)k, and (Al2S3)k-, where an unit of Al2S3 aggregates with ion cores of AlS-, AlS2-, and Al2S3, respectively. Al3S3 is exceptionally stable with its geometrical structure.

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